Big difference between upping the final drive ratio by changing one or other sprocket, and changing the ratios on individual gears . . . not quite sure what you're aiming for here Chris!
I don't know how many crank- or final drive-teeth one of these engines will comfortably pull in top, but received wisdom is that standard top gear is good, mostly. However, I've upped my final drive sprocket by one tooth on my A10, because I happen to live in the back of beyond and it's nice to cruise along at stress-free rpm when acceleration isn't the be-all-and-end-all. With rear sets you can probably put anything on the gearbox (you can't with the standard foot rests, that's for sure) while changing the crankshaft sprocket is the other, more expensive, option. An extra tooth on the final drive sprocket makes main road cruising at 65-70mph relatively relaxed, but motorways are still a slow-lane business these days.
However, if I have a complaint about the STD BSA box it's not top, it's second. It's too low. OK in traffic etc, but for me, too big a gap up and down to third. Changing sprockets obviously can't help there. An RRT2 cluster requires a lot of clutch slip in first, as I recall, and that's not great either. Not to mention the other changes that go with. I just live with what I think is too low a second gear for a country bumpkin.
A 5-speed (if money no object?)?